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Chen Chao-Yue Qiao Yu Zhang Lei Wang Xin Yang Ting-Hai 《Research on Chemical Intermediates》2020,46(9):4079-4089
Research on Chemical Intermediates - When synthesizing cyclohexane-annulated pyrazolones from a cyclohexonedicarboxylate derivative with phenylhydrazine under the catalysis of sulfuric acid in the... 相似文献
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International Journal of Theoretical Physics - The Majorana representation, which provides an intuitive way to represent the quantum state by stars on the Bloch sphere, has drawn considerable... 相似文献
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石墨相氮化碳(g?C3N4)由于具有对可见光吸收范围较窄和光生载流子分离效率低等缺陷,其光解水产氢活性较差。我们采用简单的一步热共聚法,以尿素和2,4,6?三氨基嘧啶(TAPD)混合物为前驱物,制备碳自掺杂纳米片(CNNS?x,x mg代表掺入TAPD的质量)。X射线衍射(XRD)、元素分析(EA)和X射线光电子能谱(XPS)等测试结果表明,来自TAPD的嘧啶环成功引入g?C3N4共轭体系中,使所得的CNNS?x具有较窄的带隙,较快的光生载流子迁移速率,从而提高其对可见光的吸收效率和光生载流子的分离效率。得益于此,CNNS?x在可见光照射下表现出较好的光解水产氢活性。特别是CNNS?30具有最佳光解水性能,其产氢速率可达57.6μmol·h-1,是g?C3N4纳米片(CNNS)的4倍。 相似文献
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In this paper, bifurcation trees of periodic motions in a periodically forced, time-delayed, hardening Duffing oscillator are analytically predicted by a semi-analytical method. Such a semi-analytical method is based on the differential equation discretization of the time-delayed, nonlinear dynamical system. Bifurcation trees for the stable and unstable solutions of periodic motions to chaos in such a time-delayed, Duffing oscillator are achieved analytically. From the finite discrete Fourier series, harmonic frequency-amplitude curves for stable and unstable solutions of period-1 to period-4 motions are developed for a better understanding of quantity levels, singularity and catastrophes of harmonic amplitudes in the frequency domain. From the analytical prediction, numerical results of periodic motions in the time-delayed, hardening Duffing oscillator are completed. Through the numerical illustrations, the complexity and asymmetry of period-1 motions to chaos in nonlinear dynamical systems are strongly dependent on the distributions and quantity levels of harmonic amplitudes. With the quantity level increases of specific harmonic amplitudes, effects of the corresponding harmonics on the periodic motions become strong, and the certain complexity and asymmetry of periodic motion and chaos can be identified through harmonic amplitudes with higher quantity levels. 相似文献
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Ontology is a semantic analysis and calculation model, which has been applied to many subjects. Ontology similarity calculation and ontology mapping are employed as machine learning approaches. The purpose of this paper is to study the leave-two-out stability of ontology learning algorithm. Several leave-two-out stabilities are defined in ontology learning setting and the relationship among these stabilities are presented. Furthermore, the results manifested reveal that leave-two-out stability is a sufficient and necessary condition for ontology learning algorithm. 相似文献
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To solve the target covering problems in three-dimensional space, putting forward a deployment strategies of the target points innovatively, and referencing to the differential evolution (DE) algorithm to optimize the location coordinates of the sensor nodes to realize coverage of all the target points in 3-D surface with minimal sensor nodes. Firstly, building the three-dimensional perception model of sensor nodes, and putting forward to the blind area existing in the process of the sensor nodes sensing the target points in 3-D surface innovatively, then proving the feasibility of solving the target coverage problems in 3-D surface with DE algorithm theoretically, and reflecting the fault tolerance of the algorithm. 相似文献
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Considering the importance of damage for the structural performance and for decreasing the identification error, this paper proposes an optimal sensor placement method based on a weighted standard deviation norm (WSDN) index. The standard deviation of the identified damage parameters is solved using the series expansion theory and probabilistic method to quantify the effect of a measurement error on damage identification. The damage estimation weight (DEW) index, which can reflect the importance of each element in the structural capabilities, is established based on a performance-damage curve. A significant DEW for a specified element indicates that the element is important for the structure and that its identification error should be small. The WSDN index is obtained from the Hadamard product of the standard deviations (SDs) and DEWs. Thus, the identification error of the entire structure is measured using the weighting coefficient. The optimal sensor placement (OSP) procedure is performed by minimizing the WSDN index. The proposed method can clearly decrease the uncertainties of the identification results for the important elements. Other OSP criteria, including the condition number, information entropy, and standard deviation norm, which aim to decrease the identification error, are discussed in this paper for comparison with the proposed method. Two numerical examples and an experiment, which pertain to the deformation performance, buckling features, and dynamic characteristics, are discussed to verify the advantages of the proposed method. 相似文献
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Our main goal in the present work is to address an integro-differential model under localized viscoelastic and frictional effects arising in the Boltzmann theory of viscoelasticity. More precisely, we consider a general version in the history context of the pioneer localized viscoelastic problem approached by Cavalcanti and Oquendo (2003) in the null history scenario, and more recently by Cavalcanti et al. (2018) in the history framework. By means of a new observability inequality, we prove a general stability result to the model under a weaker assumption on the localized frictional damping and a slower condition on the decreasing memory kernel (of polynomial type) than the previously mentioned works. To achieve such stability results, we still work in a general setting by removing the assumption on complementary damping mechanisms and show, in some reasonable situations concerning the density coefficient, that the localized viscoelastic effect is enough to ensure the general stability (of polynomial type) to the problem. 相似文献